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Porous crystalline materials, such as metal-organic frameworks, possess ordered internal structures that can selectively host and transport molecules. Their performance in applications such as separations, catalysis, and storage depends strongly on how they are assembled. Our research examines how molecular interactions, topology, and processing conditions influence the formation and stability of porous crystals. Rather than focusing solely on idealized structures, we aim to understand realistic assembly pathways and failure modes. This perspective helps bridge the gap between theoretical design and experimental realization. Ultimately, we seek general principles that can guide the reliable creation of functional porous materials.